NERC-funded fellowship project: The influence of surfactants on the mechanisms of ocean bubble generation and the consequences for air-sea gas transfer

The bubble clouds formed underneath breaking waves have been shown to have a significant influence on air-sea gas transfer rates, and current models for bubble clouds exist. However, no models to date have included the changes to the bubble population caused by surfactants, and consequently the total effect of surfactants on gas transfer rates. The fellowship research proposed here will build such a model, based on insights into bubble dynamics resulting from laboratory, wave tank and oceanic experimental work.
There is strong evidence to suggest that bubbles scavenge natural surfactants very quickly: the rapid reformation of the surface microlayer after an ocean wave breaks is mediated by larger bubbles bringing surfactants up to the surface and optical scattering evidence suggests that most small bubbles are coated in surfactant. To date, very few studies have considered the details of how surfactants could affect bubble formation dynamics underneath breaking waves (particularly fragmentation and coalescence), although surfactants have been shown to influence bubble dynamics. However, an understanding of the mechanistic origin of ocean bubbles is essential to guide effective parameterizations of any upper ocean process affected by bubbles.
This project will begin with laboratory studies of the effects of various natural and artificial surfactants on fragmentation and coalescence events. Simultaneous high-speed photography and acoustics have been shown to produce an impressive amount of information about individual events, and these techniques will be combined to study the dynamics and acoustics of fragmentation and coalescence events. In the second and third years of the project, the insights gained from the small-scale laboratory experiments will be used to tune models of the bubbles produced by breaking waves with different surfactants present, and these model outcomes will be tested in a wave tank and at sea.

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Detailed dynamics of bubble production by raindrops.
Last year a large dataset of stereo high-speed photography accompanied by the simultaneous acoustical signals was gathered for the bubbles generated by fresh raindrops falling on seawater. The surfactants present in the tank were varied, and we are looking for changes that these surfactants may cause in the bubbles produced. The data was collected at SIO with the help of Grant Deane and Dale Stokes, and preliminary analysis of this data is being undertaken by my intern, James Wallis.